Search for: All records

Abstract Achieving efficient and stable blue light‐emitting perovskite nanocrystals is a significant challenge for next‐generation optoelectronic devices. Here, a dual‐ligand surface engineering strategy is reported for quasi‐2D CsPbBr₃nanoplatelets (NPLs) synthesized via ligand‐assisted reprecipitation. By synergistically co‐introducing didodecyldimethylammonium bromide to passivate bromine vacancies and hexylphosphonic acid to bind undercoordinated lead ions, the NPLs achieved a remarkable photoluminescence quantum yield of 93.7% and a narrow full‐width at half‐maximum of 19.27 nm. The enhanced photoluminescence (PL) lifetime (6.35 ns), reduced crystal disorder, slower bleach recovery kinetics, and improved thermal stability suggest that the suppressed non‐radiative pathways and strong exciton confinement (Eb = 141.76 meV) result from effective surface defect passivation and enhanced radiative recombination. Additionally, surface and structural characterizations confirmed the successful dual‐ligand integration and improved crystal integrity. The treated NPLs retained ∼57% PL under 450 min of ultraviolet (UV) light and ∼55% PL under 70% relative humidity, demonstrating strong UV and moisture stability. A prototype white light‐emitting device fabricated by integrating dual‐ligand‐treated NPLs achieves a wide color gamut (121% National Television System Committee, 90.4% ITU‐R Recommendation BT.2020), demonstrating their potential for high‐performance optoelectronics. This approach promotes defect suppression in low‐dimensional perovskites, paving the way for stable and efficient blue emitters. 

We prepare quasi-1D films of Sb2Se3 on GaAs by molecular beam epitaxy. The aligned grains and anisotropic bonding hierarchy of the Sb2Se3 unit cell together produce giant birefringence in the near-infrared. 

Sub-wavelength diffractive meta-optics have emerged as a versatile platform to manipulate light fields at will, due to their ultra-small form factor and flexible multifunctionalities. However, miniaturization and multimodality are typically compromised by a reduction in imaging performance; thus, meta-optics often yield lower resolution and stronger aberration compared to traditional refractive optics. Concurrently, computational approaches have become popular to improve the image quality of traditional cameras and exceed limitations posed by refractive lenses. This in turn often comes at the expense of higher power and latency, and such systems are typically limited by the availability of certain refractive optics. Limitations in both fields have thus sparked cross-disciplinary efforts to not only overcome these roadblocks but also to go beyond and provide synergistic meta-optical–digital solutions that surpass the potential of the individual components. For instance, an application-specific meta-optical frontend can preprocess the light field of a scene and focus it onto the sensor with a desired encoding, which can either ease the computational load on the digital backend or can intentionally alleviate certain meta-optical aberrations. In this review, we introduce the fundamentals, summarize the development of meta-optical computational imaging, focus on latest advancements that redefine the current state of the art, and give a perspective on research directions that leverage the full potential of sub-wavelength photonic platforms in imaging and sensing applications. The current advancement of meta-optics and recent investments by foundries and technology partners have the potential to provide synergistic future solutions for highly efficient, compact, and low-power imaging systems. 

Abstract Silicon is a common material of choice for semiconductor optics in the infrared spectral range, due to its low cost, well-developed high-volume manufacturing methods, high refractive index, and transparency. It is, however, typically ill-suited for applications in the visible range, due to its large absorption coefficient, especially for green and blue light. Counterintuitively, we demonstrate how ultra-thin crystalline meta-optics enable full-color imaging in the visible range. For this purpose, we employ an inverse design approach, which maximizes the volume under the broadband modulation transfer function of the meta-optics. Beyond that, we demonstrate polarization-multiplexed functionality in the visible. This is particularly important as polarization optics require high index materials, a characteristic often difficult to obtain in the visible. 

Abstract Metalenses, with their ultrathin thicknesses and their ease for achieving ultra small diameters, offer a promising alternative to refractive lenses in miniaturized imaging systems, such as endoscopes, potentially enabling applications in tightly confined spaces. However, traditional metalenses suffer from strong chromatic aberrations, limiting their utility in multi-color imaging. To address this limitation, here we present an inverse-designed polychromatic metalens with a diameter of 680 μm, focal length of 400 μm, and low dispersion across 3 distinct wavelengths at 643 nm, 532 nm, and 444 nm. The metalens collimates and steers light emitted from a scanning fiber tip, generating scanning beams across a 70° field-of-view to provide illumination for a scan-based imaging. The metalens provides a close-to-diffraction-limited 0.5° angular resolution, only restricted by the effective aperture of the system. The average relative efficiency among three design wavelengths is around 32% for on-axis angle and 13% averaged across the entire field-of-view. This work holds promise for the application of metalenses in endoscopes and other miniaturized imaging systems. 

Programmable photonic integrated circuits are expected to play an increasingly important role in enabling high-bandwidth optical interconnects and large-scale in-memory computing as needed to support the rise of artificial intelligence and machine learning technology. To that end, chalcogenide-based non-volatile phase-change materials (PCMs) present a promising solution due to zero static power. However, high switching voltage and a small number of operating levels present serious roadblocks to the widespread adoption of PCM-programmable units. Here, we demonstrate an electrically programmable wide bandgap Sb2S3-clad silicon ring resonator using a silicon microheater at a complementary-metal–oxide–semiconductor compatible voltage of <3 V. Our device shows a low switching energy of 35.33 nJ (0.48 mJ) for amorphization (crystallization) and reversible phase transitions with high endurance (>2000 switching events) near 1550 nm. Combining a volatile thermo-optic effect with non-volatile PCMs, we demonstrate 7-bit (127 levels) operation with excellent repeatability and reduced power consumption. Our demonstration of low-voltage and low-energy operation, combined with the hybrid volatile–nonvolatile approach, marks a significant step toward integrating PCM-based programmable units in large-scale optical interconnects.